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Pure Appl. Chem., 2009, Vol. 81, No. 7, pp. 1217-1227

http://dx.doi.org/10.1351/PAC-CON-08-10-08

Published online 2009-05-29

Scorpionate complexes of vanadium(III or IV) as catalyst precursors for solvent-free cyclohexane oxidation with dioxygen

Gopal S. Mishra1, Telma F. S. Silva2,1, Luísa M. D. R. S. Martins1,3 and Armando J. L. Pombeiro1*

1 Centro de Química Estrutural, Complexo I, Instituto Superior Técnico, TU Lisbon, Av. Rovisco Pais, 1049-001, Lisbon, Portugal
2 Área Científica de Física, ISEL, R. Conselheiro Emídio Navarro, 1959-007, Lisbon, Portugal
3 Departamento de Engenharia Química, ISEL, R. Conselheiro Emídio Navarro, 1959-007, Lisbon, Portugal

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  • Fernandes Ricardo R., Lasri Jamal, da Silva M. Fátima C. Guedes, da Silva José A.L., Fraústo da Silva João J.R., Pombeiro Armando J.L.: Mild alkane C–H and O–H oxidations catalysed by mixed-N,S copper, iron and vanadium systems. CATAL A GENERAL 2011, 402, 110. <http://dx.doi.org/10.1016/j.apcata.2011.05.035>
  • Silva Telma F.S., Guedes da Silva M. Fátima, Mishra Gopal S., Martins Luísa M.D.R.S., Pombeiro Armando J.L.: Synthesis and structural characterization of iron complexes with 2,2,2-tris(1-pyrazolyl)ethanol ligands: Application in the peroxidative oxidation of cyclohexane under mild conditions. J Organomet Chem 2011, 696, 1310. <http://dx.doi.org/10.1016/j.jorganchem.2010.12.036>
  • Fernandes Ricardo R., Lasri Jamal, Guedes da Silva M. Fátima C., da Silva José A.L., Fraústo da Silva João J.R., Pombeiro Armando J.L.: Bis- and tris-pyridyl amino and imino thioether Cu and Fe complexes. Thermal and microwave-assisted peroxidative oxidations of 1-phenylethanol and cyclohexane in the presence of various N-based additives. Journal of Molecular Catalysis A 2011, 351, 100. <http://dx.doi.org/10.1016/j.molcata.2011.09.022>
  • Marchetti Fabio, Pettinari Claudio, Pettinari Riccardo, Cerquetella Adele, Martins Luísa M. D. R. S., Guedes da Silva M. Fátima C., Silva Telma F. S., Pombeiro Armando J. L.: Ruthenium(II) Arene Complexes Bearing Tris(pyrazolyl)methanesulfonate Capping Ligands. Electrochemistry, Spectroscopic, and X-ray Structural Characterization. Organomettalics 2011, 30, 6180. <http://dx.doi.org/10.1021/om200713v>
  • Silva Telma F. S., Luzyanin Konstantin V., Kirillova Marina V., da Silva M. Fátima Guedes, Martins Luísa M. D. R. S., Pombeiro Armando J. L.: Novel Scorpionate and Pyrazole Dioxovanadium Complexes, Catalysts for Carboxylation and Peroxidative Oxidation of Alkanes. Adv Synth Catal 2010, 352, 171. <http://dx.doi.org/10.1002/adsc.200900660>
  • Silva Telma F. S., Mishra Gopal S., Guedes da Silva M. Fátima, Wanke Riccardo, Martins Luísa M. D. R. S., Pombeiro Armando J. L.: CuII complexes bearing the 2,2,2-tris(1-pyrazolyl)ethanol or 2,2,2-tris(1-pyrazolyl)ethyl methanesulfonate scorpionates. X-Ray structural characterization and application in the mild catalytic peroxidative oxidation of cyclohexane. Dalton Trans 2009, 9207. <http://dx.doi.org/10.1039/b911990f>